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I see alot of shirt with designs on them that look like diamonds. I example I saw a t shirt with 2PAC on it and he was wearing a cross that looked liked it was made of diamonds and gold (bling). Where can I get that from and what type of material is that?
there are metallic pantone spot colors that can be used such as 871, 872 & other "800's". there are also metallic foils that are used to create that type of effect. check with your local screenprinter to see what they offer.
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Diamond, Gold, Platium effect...? 
